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All 9 seasons in 720p, the Movie, most of Equestria Girls (might be missing a short or two, and waiting for a full cut of Backstage Pass).
I'm behind on the comics and still waiting for a non-broadcast version of Rainbow Roadtrip. But once it's all saved, I'm going to burn to BD-R disks where they will be preserved for all eternity.
Maybe I should start backing up all my fimfiction bookshelves in case that treasure trove ever goes down.